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| Episode Information | |||
| The When in Rome Affair | |||
| Cast | Crew | ||
| Sid Haig | Vito | George Waggner | Director |
| Robert Vaught | Napoleon Solo | Gloria Elmore | Writer |
| David McCallum | Illya Kuryakin | Irv Pearlberg | Producer |
| Leo Carroll | Mr. Alexander Waverly | Norman Felton | Executive Producer |
| Julie Sommars | Darlene Sims | David Victor | Supervising Producer |
| Cesare Danova | Count Cesare Guardia | Jerry Goldsmith | Theme Music |
| Kathleen Freeman | Mrs. Sparks | Robert Drasnin | Original Music |
| Than Wyenn | Bruno | ||
| Bill Corcoran | Sammy Sparks | ||
| Stuart Nisbet | George Sparks | ||
| Sharyn Hillyer | Wanda | ||
| Benito Prezia | Bus Driver | ||
| Franco Corsaro | Clerk | ||
| The Prince of Darkness Affair: Part I | |||
| Cast | Crew | ||
| Sid Haig | Alex | Boris Sagal | Director |
| Robert Vaught | Napoleon Solo | Dean Hargrove | Writer |
| David McCallum | Illya Kuryakin | Irv Pearlberg | Producer |
| Leo Carroll | Mr. Alexander Waverly | Norman Felton | Executive Producer |
| Carol Lynley | Annie Justin | David Victor | Supervising Producer |
| Bradford Dillman | Luther Sebastian | Jerry Goldsmith | Theme Music |
| Lola Albright | Azalea | Robert Drasnin | Original Music |
| John Dehner | Dr. Parviz Kharmusi | ||
| John Carradine | Old Man | ||
| H.M. Wynant | Hassan Askoy | ||
| Roy Jenson | Carl | ||
| Arthur Malet | White Hunter | ||
| Robert Karnes | Captain | ||
| Mort Thompson | Henchman | ||
| Barbara Moore | Lisa Rogers | ||